Design of van der Waals interfaces for broad-spectrum optoelectronics

Two-Dimensional Semiconductor Optoelectronics Based on van der Waals Heterostructures

Two-dimensional (2D) semiconductors such as transition metal dichalcogenides (TMDCs) and black phosphorous have drawn tremendous attention as an emerging optical material due to their unique and remarkable optical properties. In addition, the ability to create the atomically-controlled van der Waals (vdW) heterostructures enables realizing novel optoelectronic devices that are distinct from con...

Van der Waals interactions with soft interfaces

Many naturally occurring microbiological and synthetic polymer systems have soft interfaces due, e.g., to the presence of polymer brushes at the surfaces. The initial interactions (before contact) in such systems are typically physical rather than chemical in origin, e.g. electrostatic or van der Waals forces. We calculate the form of the summed van der Waals interaction energies UHS and USS be...

Correction to "charge transfer excitons at van der Waals interfaces".

The van der Waals interfaces of molecular donor/acceptor or graphene-like two-dimensional (2D) semiconductors are central to concepts and emerging technologies of light-electricity interconversion. Examples include, among others, solar cells, photodetectors, and light emitting diodes. A salient feature in both types of van der Waals interfaces is the poorly screened Coulomb potential that can g...

Supporting Information Near-Unity Absorption in Van der Waals Semiconductors for Ultrathin Optoelectronics

Near-Unity Absorption in van der Waals Semiconductors for Ultrathin Optoelectronics.

We demonstrate near-unity, broadband absorbing optoelectronic devices using sub-15 nm thick transition metal dichalcogenides (TMDCs) of molybdenum and tungsten as van der Waals semiconductor active layers. Specifically, we report that near-unity light absorption is possible in extremely thin (<15 nm) van der Waals semiconductor structures by coupling to strongly damped optical modes of semicond...